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Portman has been a vegetarian since childhood^[28] and is an advocate for animal rights. She does not eat animal products or wear fur, feathers or leather. "All of my shoes are from Target and Stella McCartney", she says.^[29] oguztoydemir It has been reported that she will appear alongside actress Elissa Sursara in a PETA PSA to support the groups anti-fur campaign at some point throughout 2009.^[30] In 2007, Natalie Portman traveled to Rwanda with Jack Hanna, to film a documentary titled Gorillas on the Brink. Later at a naming ceremony, Portman named a baby gorilla Gukina, which means 'to play'.^[31] In 2007, she launched her own brand of vegan footwear.^[32] Portman has been an advocate of environmental causes since childhood, when she joined an environmental song and dance troupe known as World Patrol Kids.^[33]

Portman has been involved with the 2004 presidential campaign of Democratic candidate John Kerry and with antipoverty activities. In 2004 and 2005 she traveled to Uganda, Guatemala, and Ecuador as the Ambassador of Hope for FINCA International, an organization that promotes micro-lending to help finance women-owned businesses in poor countries.^[34] In an interview conducted backstage at the Live 8 concert in Philadelphia and appearing on the PBS program Foreign Exchange with Fareed Zakaria she discussed microfinance.^[35] Host Fareed Zakaria said that he was "generally wary of celebrities with fashionable causes", but included the segment with Portman because "she really knew her stuff".^[36] In the "Voices" segment of the April 29, 2007, episode of the ABC Sunday Morning Program This Week with George Stephanopoulos, Portman discussed her work with FINCA and how it can benefit women and their children in third world countries.^[37] In the Fall of 2007, Portman visited several university campuses, including Harvard, UCLA, UC Berkeley, Stanford, Princeton, New York University, and Columbia, to inspire students with the power of microfinance and to encourage them to join the Village Banking Campaign to help families and communities lift themselves out of "nicole kidman" "transparent dress" poverty.^[38]

Portman has commented on V for Vendetta's political relevance, and mentioned that her character, who joins an underground anti-government group, is "often bad and does things that you don't like" and that "Being from Israel was a reason I wanted to do this because terrorism and violence are such a daily part of my conversations since I was little." She said the film "doesn't make clear good or bad statements. It respects the audience enough to take away their own opinion".^[62] Search Both Goya's Ghosts and Free Zone received limited releases in 2006. Portman starred in the children's film Mr. Magorium's Wonder Emporium, which began filming in April 2006 and was released in November 2007; she has said that she was "excited to do a kids' movie."^[60] In late 2006, Portman filmed The Other Boleyn Girl, a historical drama in which she plays Anne Boleyn; Eric Bana and Scarlett Johansson co-starred in the film. She was also named one of the hottest women of film and TV by Blender Magazine.^[63]